Chromatography for protein separation

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Size exclusion: large first. Ion exchange: opposite charges bind. Affinity: the matching target binds.

Size exclusion: access to pores

Size exclusion chromatography (SEC) uses porous beads. Large molecules enter fewer pores and take a shorter route through the column, so they elute first. Smaller molecules explore more pore volume and elute later. Separation reflects hydrodynamic size, so shape also matters. SEC is useful for separating aggregates, exchanging buffers, and estimating size under calibrated conditions.

Large particles bypass bead pores and emerge first; smaller particles enter pores and emerge later.
Size exclusion chromatography ResearchGate figure credited in the Khan Academy source · Source attribution · Original image ↗

Ion exchange: opposite charges attract

  • Anion exchange uses a positively charged resin, such as DEAE, to bind negative proteins. Cation exchange uses a negatively charged resin to bind positive proteins.
  • At pH above its pI, a protein is net negative; below its pI, it is net positive. Choose the buffer and resin together.
  • Unbound proteins pass through. Increasing salt competes with charge interactions; changing pH changes protein charge. Either can release bound proteins.
Positively charged DEAE resin binds negative proteins at low salt and releases them as salt concentration increases.
Ion exchange chromatography ScienceDirect, as credited by Khan Academy · Source attribution · Original image ↗

Affinity: selective binding

Affinity chromatography captures a target with an immobilized binding partner. Wash away unbound material, then release the target with a competing ligand or altered conditions. Examples include antibody–antigen binding, His-tag binding to metal-containing resin, and GST-tag binding to glutathione.

A target binds an immobilized ligand, unbound material is washed away, and the bound target is released.
Affinity chromatography Khan Academy · CC BY-NC-SA 4.0 · Original image ↗

Gas chromatography

GC uses an inert carrier gas, a heated column, and a detector. In GLC, the stationary phase is a liquid film; in GSC, it is a solid. Retention depends on volatility and stationary-phase interactions. Detector options include FID, TCD, ECD, and MS. GC suits volatile, thermally stable compounds; intact proteins generally require liquid-phase methods rather than direct GC.

Carrier gas moves an injected sample through a column in an oven to a detector.
Gas chromatography apparatus Khan Academy · CC BY-NC-SA 4.0 · Original image ↗

High performance liquid chromatography

HPLC uses high-pressure pumps and efficient packed columns. The stationary phase determines what separates the sample: HPLC is not itself a single separation mechanism. RP-HPLC has a nonpolar stationary phase and commonly separates peptides by hydrophobic interactions. NP-HPLC uses a polar stationary phase.

Solvent is pumped through an injection system and column to a detector and output.
HPLC apparatus Khan Academy · CC BY-NC-SA 4.0 · Original image ↗

The detector records a chromatogram of signal against retention time. UV-visible absorbance, RID, and MS are possible detection methods. A peak’s position helps identification under validated conditions; its area supports quantification with suitable calibration.

29 terms, alphabetically ordered

Affinity chromatography
Separation by specific binding between a target and an immobilized ligand, followed by selective release.
Anion exchangeanion exchanger
A method using positively charged resin to bind negatively charged molecules.
Antibodyantibodies
An immune protein that specifically binds a molecular target called an antigen.
Cation exchangecation exchanger
A method using negatively charged resin to bind positively charged molecules.
Chromatography
Separation of mixture components by their different interactions with a stationary phase and a moving mobile phase.
DiethylaminoethylDEAE
A positively charged functional group used in anion-exchange resins, such as DEAE-cellulose.
Electron capture detectorECD
A gas chromatography detector sensitive to substances that capture electrons, such as many halogenated compounds.
Elutionelute · eluted
Removal of a component from the stationary phase by the flowing mobile phase.
Flame ionization detectorFID
A gas chromatography detector that measures ions generated when organic compounds burn in a flame.
Gas chromatographyGC
Separation of volatile, thermally stable compounds carried through a column by a gas. Retention depends on volatility and stationary-phase interactions.
Gas-liquid chromatographyGLC
Gas chromatography with a liquid stationary-phase film and a gaseous mobile phase.
Gas-solid chromatographyGSC
Gas chromatography with a solid adsorbent stationary phase and a gaseous mobile phase.
Glutathione S-transferaseGST · GST-tag
An enzyme used as a fusion tag; GST-tagged proteins can bind a glutathione affinity matrix.
High performance liquid chromatographyHPLC · high-performance liquid chromatography
Liquid chromatography using high-pressure pumps and an efficient packed column. The separation mechanism depends on the stationary phase.
Histidine tagHis-tag
A short chain of histidines added to a protein to enable purification on an immobilized metal-affinity resin.
Hydrophobic
Interacting poorly with water. Nonpolar side chains often gather in a soluble protein’s interior.
Ion exchange chromatographyIEX · ion-exchange chromatography
Separation by net charge through reversible binding to an oppositely charged resin.
Isoelectric pointpI · isoelectric points
The pH at which a molecule has zero net electrical charge. In isoelectric focusing, a protein accumulates where local pH equals its pI.
Mass spectrometryMS · mass spectrometer
Analysis of ionized molecules according to their mass-to-charge ratios, used to identify and quantify proteins or peptides.
Mobile phasecarrier
The moving fluid that carries a sample through a chromatographic system.
Normal-phase HPLCNP-HPLC
High performance liquid chromatography with a polar stationary phase and less polar mobile phase.
pH
A measure of acidity, defined as the negative base-10 logarithm of hydrogen ion activity. Lower pH means greater acidity; pH influences amino acid charge.
Refractive index detectorRID
A chromatography detector that measures changes in refractive index when analytes pass through it.
Retention timeretention times
The elapsed time between sample injection and detection of a component leaving the column.
Reversed-phase HPLCRP-HPLC · reverse-phase HPLC
High performance liquid chromatography with a nonpolar stationary phase and polar mobile phase.
Size exclusion chromatographySEC · size-exclusion chromatography · gel filtration chromatography
Separation by hydrodynamic size using porous beads. Large molecules access fewer pores and usually elute before small molecules.
Stationary phaseadsorbent
The material that remains fixed in a chromatographic system.
Thermal conductivity detectorTCD
A gas chromatography detector that measures changes in thermal conductivity of the carrier gas.
Ultraviolet-visible detectionUV-visible · UV-Vis
Measurement of light absorbance at ultraviolet or visible wavelengths as compounds leave a chromatography column.

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